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Renfe
The train service in Spain is excellent, especially the high speed trains (AVEs) which run between most of the main cities. If you are taking the high speed rail service elsewhere the local leg (cercania) of the journey is free. The Renfe website gives timetables and allows you to book online. If you're over 60, it's worth getting a Tarjeta Dorada for great discounts. The card costs just €6 and is valid for a year.
This website is really useful if you're trying to book rail travel within Spain.
Trainline
Trainline is the leading train and bus ticket company in Europe with information about routes, fares and travel schedules from 270 train and bus operators in 45 countries, so that everyone can buy tickets quickly, saving time and money and avoiding setbacks. By purchasing your train tickets with Trainline, you can get fantastic discounts. Find out here about the discounts you are entitled to and benefit from travelling more by train for much less.
We hope to provide more useful booking links soon!